As you progress in the game, the police chief will steadily deploy more and more police officers to the streets in their stupid little golf carts. There's no need to make a specific effort to unlock this achievement, as sooner or later you'll need to destroy a cop car in order to get away to return a Jinjo or just get them off your back after accidentally bumping into them while returning a crate. Destroy any of these cop carts to pop the achievement.